Graphitic carbon nitride-based z-scheme structure for photocatalytic CO2 reduction
Document Type
Journal Article
Publication Title
Energy and Fuels
Volume
35
Issue
1
First Page
7
Last Page
24
Publisher
American Chemical Society Publications
School
School of Engineering
RAS ID
32847
Funders
Australian Research Council
Grant Number
ARC Number : DP170104264
Grant Link
http://purl.org/au-research/grants/arc/DP170104264
Abstract
© Photocatalytic CO2 reduction (PCR) into hydrocarbon fuels and chemicals such as CH4, CH3OH, HCHO, and HCOOH is a promising strategy for simultaneously solving environmental challenges and realizing solar-to-energy conversion for sustainable development. Among the photocatalysts developed, graphitic carbon nitride (g-C3N4, GCN) is widely applied in PCR, ascribing to its suitable electronic and physicochemical attributes. In the enhancement of the photocatalytic activity of GCN in PCR, substantial efforts have been made by coupling GCN with auxiliary semiconductors to construct direct or indirect Z-scheme structures using effective methods. Aiming to offer insights into structure-activity relationships, we summarize the latest advancements in the GCN-based Z-scheme structure (ZSS) in this review, with respect to the structure engineering strategies for direct ZSS construction and various approaches for indirect ZSS configuration. The present issues and perspectives of GCN-based ZSS for PCR are also presented and discussed.
DOI
10.1021/acs.energyfuels.0c03048
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Comments
Lin, J., Tian, W., Zhang, H., Duan, X., Sun, H., & Wang, S. (2021). Graphitic carbon nitride-based z-scheme structure for photocatalytic CO2 reduction. Energy & Fuels, 35(1), 7-24. https://doi.org/10.1021/acs.energyfuels.0c03048